We have investigated the performance of some important simplifying approximations in ion–polyatom scattering. It is shown that a simple linearly forced harmonic oscillator model combined with an anharmonic projection offers a sufficiently accurate description of proton energy loss spectra in H+–CF4 collisions if the CF4 molecule is excited from the vibrational ground state.
G. D. Billing, J. Chem. Soc., Faraday Trans., 1990, 86, 1663 DOI: 10.1039/FT9908601663
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