Benzene-induced 1H n.m.r. shifts reported for a variety of polar solutes are related to the magnitude of the solute dipole moment for groups of structurally similar molecules. N.m.r. and Kerr constant data are interpreted in terms of a time-averaged solvent cluster model; the most favoured stereospecific solute–benzene interactions within the solvation sphere are indicated.
R. S. Armstrong, M. J. Aroney, R. K. Duffin, H. J. Stootman and R. J. W. Le Fèvre, J. Chem. Soc., Perkin Trans. 2, 1973, 1272 DOI: 10.1039/P29730001272
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