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Issue 2, 2015
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Crystallization and concentration modulated tunable upconversion luminescence of Er3+ doped PZT nanofibers

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Abstract

Ferroelectric oxides with excellent electrical, mechanical and optical multifunctions play a vital role in future microdevices with diverse applications in energy, sensors and actuators. A series of Er doped PbZr0.52Ti0.48O3 (PZT:Er3+) nanofibers with tunable upconversion photoluminescence (PL) properties were successfully synthesized via a sol–gel based electrospinning process. By controlled crystallization, PZT:Er3+ nanofibers evolve from a polycrystalline to a single-crystalline-like structure, resulting in a remarkable increase in the visible upconversion emission intensity. It was uncovered that Er3+ doping site in PZT shifts from B site to A site with increase in crystallinity and crystal size. In addition, remarkable enhancement in red emission is observed with increased Er3+ doping concentration, which facilitates the modulation of emission colour from green to orange. Combined with the excellent ferroelectric properties of PZT, such spectral tunable PZT:Er3+ nanofibers are considered as a promising multifunctional candidate for integrated electro-mechano-optical devices.

Graphical abstract: Crystallization and concentration modulated tunable upconversion luminescence of Er3+ doped PZT nanofibers

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Supplementary files

Article information


Submitted
12 Aug 2014
Accepted
29 Oct 2014
First published
31 Oct 2014

J. Mater. Chem. C, 2015,3, 382-389
Article type
Paper

Crystallization and concentration modulated tunable upconversion luminescence of Er3+ doped PZT nanofibers

Y. Fu, S. Gong, X. Liu, G. Xu, Z. Ren, X. Li and G. Han, J. Mater. Chem. C, 2015, 3, 382
DOI: 10.1039/C4TC01784F

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