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Issue 33, 2020
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Collective motion of chiral Brownian particles controlled by a circularly-polarized laser beam

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Abstract

We demonstrate the emergence of circular collective motion in a system of spherical light-propelled Brownian particles. Light-propulsion occurs as consequence of the coupling between the chirality of polymeric particles – left (L)- or right (R)-type – and the circularly-polarized light that irradiates them. Irradiation with light that has the same helicity as the particle material leads to a circular cooperative vortical motion between the chiral Brownian particles. In contrast, opposite circular-polarization does not induce such coupling among the particles but only affects their Brownian motion. The mean angular momentum of each particle has a value and sign that distinguishes between chiral activity dynamics and typical Brownian motion. These outcomes have relevant implications for chiral separation technologies and provide new strategies for optical torque tunability in mesoscopic optical array systems, micro- and nanofabrication of light-activated engines with selective control and collective motion.

Graphical abstract: Collective motion of chiral Brownian particles controlled by a circularly-polarized laser beam

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Article information


Submitted
06 Dec 2019
Accepted
15 Jul 2020
First published
16 Jul 2020

Soft Matter, 2020,16, 7704-7714
Article type
Paper

Collective motion of chiral Brownian particles controlled by a circularly-polarized laser beam

R. J. Hernández, F. J. Sevilla, A. Mazzulla, P. Pagliusi, N. Pellizzi and G. Cipparrone, Soft Matter, 2020, 16, 7704
DOI: 10.1039/C9SM02404B

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