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Issue 36, 2019

Engineering multilayer chemical networks

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Abstract

Dynamic multilevel systems emerged in the last few years as new platforms to study thermodynamic systems. In this work, unprecedented fully communicated three-level systems are studied. First, different conditions were screened to selectively activate thiol/dithioacetal, thiol/thioester, and thiol/disulfide exchanges, individually or in pairs. Some of those conditions were applied, sequentially, to build multilayer dynamic systems wherein information, in the form of relative amounts of building blocks, can be directionally transmitted between different exchange pools. As far as we know, this is the first report of one synthetic dynamic chemical system where relationships between layers can be changed through network operations.

Graphical abstract: Engineering multilayer chemical networks

Supplementary files

Article information


Submitted
03 May 2019
Accepted
28 Jul 2019
First published
29 Jul 2019

This article is Open Access
All publication charges for this article have been paid for by the Royal Society of Chemistry

Chem. Sci., 2019,10, 8338-8347
Article type
Edge Article

Engineering multilayer chemical networks

M. Martinez-Amezaga, A. G. Orrillo and R. L. E. Furlan, Chem. Sci., 2019, 10, 8338 DOI: 10.1039/C9SC02166C

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