Fabrication of recyclable reduced graphene oxide/graphitic carbon nitride quantum dot aerogel hybrids with enhanced photocatalytic activity

Abstract

Recyclable photocatalysts that can efficiently respond to visible light must be developed for practical application. Herein, three-dimensional (3D) reduced graphene oxide (rGO)/graphitic carbon nitride quantum dot (CNQD) aerogel hybrids for harvesting visible light were synthesized via a hydrothermal method. The graphitic CNQDs were not only decorated on but also integrated onto the surface of rGO. The CNQDs produced photogenerated charge under visible light. 3D rGO could serve as an acceptor of the photogenerated electrons and stereoscopically facilitated the charge transfer through aerogel networks owing to its high conductivity. The ciprofloxacin removal ratio of the aerogel hybrids was about 6.1 times higher than that of bulk g-C₃N₄.