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Issue 3, 2017

Synthesis of diverse heterocycles via one-pot cascade cross-dehydrogenative-coupling (CDC)/cyclization reaction

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Abstract

A cascade Cross-Dehydrogenative-Coupling (CDC)/cyclization methodology has been developed for the synthesis of diverse scaffolds. This method can be successfully employed to prepare various heterocycles including phenanthridines, lactams, lactones and dibenzofurans via a one-pot reaction. Two directing groups were used to enhance the selectivity. Our synthetic strategy exhibits several advantages including using non-prefunctional starting material, less chemical steps and easier purification process. These heterocycle compounds may have a broad utility in the field of medicinal chemistry, materials, etc.

Graphical abstract: Synthesis of diverse heterocycles via one-pot cascade cross-dehydrogenative-coupling (CDC)/cyclization reaction

Supplementary files

Article information


Submitted
07 Sep 2016
Accepted
09 Dec 2016
First published
13 Dec 2016

Org. Chem. Front., 2017,4, 386-391
Article type
Research Article

Synthesis of diverse heterocycles via one-pot cascade cross-dehydrogenative-coupling (CDC)/cyclization reaction

C. Zhang, T. Li, L. Wang and Y. Rao, Org. Chem. Front., 2017, 4, 386 DOI: 10.1039/C6QO00522E

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