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Issue 46, 2018
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Probing the SERS brightness of individual Au nanoparticles, hollow Au/Ag nanoshells, Au nanostars and Au core/Au satellite particles: single-particle experiments and computer simulations

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Abstract

Different classes of plasmonic nanoparticles functionalized with the non-resonant Raman reporter molecule 4-MBA are tested for their SERS signal brightness at the single-particle level: gold nanoparticles, hollow gold/silver nanoshells, gold nanostars, and gold core/gold satellite particles. Correlative SERS/SEM experiments on a set of particles from each class enable the unambiguous identification of single particles by electron microscopy as well as the characterization of both their elastic (LSPR) and inelastic (SERS) scattering spectra. Experimental observations are compared with predictions from FEM computer simulations based on 3D models derived from representative TEM/SEM images. Single gold nanostars and single gold core/gold satellite particles exhibit a detectable SERS signal under the given experimental conditions, while single gold nanoparticles and single hollow gold/silver nanoshells are not detectable.

Graphical abstract: Probing the SERS brightness of individual Au nanoparticles, hollow Au/Ag nanoshells, Au nanostars and Au core/Au satellite particles: single-particle experiments and computer simulations

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Article information


Submitted
26 Jul 2018
Accepted
28 Oct 2018
First published
09 Nov 2018

Nanoscale, 2018,10, 21721-21731
Article type
Paper

Probing the SERS brightness of individual Au nanoparticles, hollow Au/Ag nanoshells, Au nanostars and Au core/Au satellite particles: single-particle experiments and computer simulations

V. Tran, C. Thiel, J. T. Svejda, M. Jalali, B. Walkenfort, D. Erni and S. Schlücker, Nanoscale, 2018, 10, 21721
DOI: 10.1039/C8NR06028B

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