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Volume 151, 2011
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In situpowder neutron diffraction study of non-stoichiometric phase formation during the hydrogenation of Li3N

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Abstract

The hydrogenation of Li3N at low chemical potential has been studied in situ by time-of-flight powder neutron diffraction and the formation of a non-stoichiometric Li4−2xNH phase and Li4NH observed. The results are interpreted in terms of a model for the reaction pathway involving the production of Li4NH and Li2NH, which subsequently react together to form Li4−2xNH. Possible mechanisms for the production of Li4NH from the hydrogenation of Li3N are discussed.

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Article information


Submitted
14 Dec 2010
Accepted
01 Feb 2011
First published
21 Jun 2011

Faraday Discuss., 2011,151, 263-270
Article type
Paper

In situ powder neutron diffraction study of non-stoichiometric phase formation during the hydrogenation of Li3N

D. J. Bull, N. Sorbie, G. Baldissin, D. Moser, M. T. F. Telling, R. I. Smith, D. H. Gregory and D. K. Ross, Faraday Discuss., 2011, 151, 263
DOI: 10.1039/C0FD00020E

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