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Issue 10, 2011
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Aerosol generation by reactive boiling ejection of molten cellulose

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The generation of primary aerosols from biomass hinders the production of biofuels by pyrolysis, intensifies the environmental impact of forest fires, and exacerbates the health implications associated with cigarette smoking. High speed photography is utilized to elucidate the ejection mechanism of aerosol particles from thermally decomposing cellulose at the timescale of milliseconds. Fluid modeling, based on first principles, and experimental measurement of the ejection phenomenon supports the proposed mechanism of interfacial gas bubble collapse forming a liquid jet which subsequently fragments to form ejected aerosol particles capable of transporting nonvolatile chemicals. Identification of the bubble-collapse/ejection mechanism of intermediate cellulose confirms the transportation of nonvolatile material to the gas phase and provides fundamental understanding for predicting the rate of aerosol generation.

Graphical abstract: Aerosol generation by reactive boiling ejection of molten cellulose

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The article was received on 02 Jun 2011, accepted on 03 Aug 2011 and first published on 06 Sep 2011

Article type: Paper
DOI: 10.1039/C1EE01876K
Citation: Energy Environ. Sci., 2011,4, 4306-4321

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    Aerosol generation by reactive boiling ejection of molten cellulose

    A. R. Teixeira, K. G. Mooney, J. S. Kruger, C. L. Williams, W. J. Suszynski, L. D. Schmidt, D. P. Schmidt and P. J. Dauenhauer, Energy Environ. Sci., 2011, 4, 4306
    DOI: 10.1039/C1EE01876K

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