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Issue 10, 2018
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Directing the mechanism of CO2 reduction by a Mn catalyst through surface immobilization

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Abstract

Immobilization of a Mn polypyridyl CO2 reduction electrocatalyst on nanocrystalline TiO2 electrodes yields an active heterogeneous system and also significantly triggers a change in voltammetric and catalytic behaviour, relative to in solution. A combination of spectroelectrochemical techniques are presented here to elucidate the mechanism of the immobilized catalyst in situ.

Graphical abstract: Directing the mechanism of CO2 reduction by a Mn catalyst through surface immobilization

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Publication details

The article was received on 20 Dec 2017, accepted on 19 Feb 2018 and first published on 19 Feb 2018


Article type: Communication
DOI: 10.1039/C7CP08537K
Phys. Chem. Chem. Phys., 2018,20, 6811-6816

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    Directing the mechanism of CO2 reduction by a Mn catalyst through surface immobilization

    J. J. Walsh, M. Forster, C. L. Smith, G. Neri, R. J. Potter and A. J. Cowan, Phys. Chem. Chem. Phys., 2018, 20, 6811
    DOI: 10.1039/C7CP08537K

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