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Issue 28, 2015
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Modelling the mobility of positive ion clusters in normal liquid helium over large pressure ranges

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Abstract

Positively charged helium clusters, also called ‘snowballs’, have been investigated within normal liquid helium. Thermodynamic state equations for ionic helium clusters in liquid helium have been developed, allowing us to discern the ‘hydrodynamic’ radius for a wide range of hydrostatic pressures and temperatures. The mobilities derived from the cluster sizes using stokes law match experimental data with unsurpassed accuracy. For low pressures the compressibility of the cluster ions was found to be distinctly larger than the compressibility of solid helium suggesting that in this pressure range clusters are fully or partially liquid.

Graphical abstract: Modelling the mobility of positive ion clusters in normal liquid helium over large pressure ranges

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Article information


Submitted
30 Apr 2015
Accepted
22 Jun 2015
First published
22 Jun 2015

Phys. Chem. Chem. Phys., 2015,17, 18535-18540
Article type
Paper
Author version available

Modelling the mobility of positive ion clusters in normal liquid helium over large pressure ranges

F. Aitken, N. Bonifaci, L. G. Mendoza-Luna and K. von Haeften, Phys. Chem. Chem. Phys., 2015, 17, 18535
DOI: 10.1039/C5CP02539G

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