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Issue 73, 2020
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Hierarchically macro–meso–microporous metal–organic framework for photocatalytic oxidation

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Abstract

The macro–meso–microporous and defective metal–organic framework constructed by transition metal Zn and 2,2′-bipyridine-5,5′-carboxylate was synthesized in CO2-expanded solvent. It shows high photocatalytic activity and selectivity for the oxidation of amines to imines under mild conditions, i.e., air as an oxidant, room temperature, and involving no photosensitizer or cocatalyst.

Graphical abstract: Hierarchically macro–meso–microporous metal–organic framework for photocatalytic oxidation

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Article information


Submitted
24 Jun 2020
Accepted
03 Aug 2020
First published
04 Aug 2020

Chem. Commun., 2020,56, 10754-10757
Article type
Communication

Hierarchically macro–meso–microporous metal–organic framework for photocatalytic oxidation

Y. Sha, J. Zhang, D. Tan, F. Zhang, X. Cheng, X. Tan, B. Zhang, B. Han, L. Zheng and J. Zhang, Chem. Commun., 2020, 56, 10754
DOI: 10.1039/D0CC04389C

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