Issue 58, 2019
From the journal:

Chemical Communications

External oxidant-free oxidation/[3+2] cycloaddition/aromatization cascade: electrochemical synthesis of polycyclic N-heterocycles†

Qiang Wang, ORCID logo ab   Ting Yuan,c   Qiang Liu,ab   Yong Xu, ORCID logo ab   Guanqun Xie,a   Xin Lv, ORCID logo c   Shujiang Ding, ORCID logo b   Xiaoxia Wang*a  and  Chen Li*a  

* Corresponding authors

a School of Environment and Civil Engineering, Dongguan University of Technology, Dongguan, P. R. China

b Department of Applied Chemistry, School of Science, Xi’an Jiaotong University, Xi’an, P. R. China

c Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Zhejiang Normal University, 688 Yingbin Road, Jinhua 321004, P. R. China

Abstract

Here, we describe an efficient and environmentally friendly synthesis of polycyclic N-heterocycles under electrochemical external oxidant-free conditions. The extent of the sequential electrochemical oxidative aromatization can be regulated with the assistance of redox mediators.

Graphical abstract: External oxidant-free oxidation/[3+2] cycloaddition/aromatization cascade: electrochemical synthesis of polycyclic N-heterocycles

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Article information

DOI
https://doi.org/10.1039/C9CC04336E
Article type
Communication
Submitted
06 Jun 2019
Accepted
19 Jun 2019
First published
19 Jun 2019

Chem. Commun., 2019,55, 8398-8401

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External oxidant-free oxidation/[3+2] cycloaddition/aromatization cascade: electrochemical synthesis of polycyclic N-heterocycles

Q. Wang, T. Yuan, Q. Liu, Y. Xu, G. Xie, X. Lv, S. Ding, X. Wang and C. Li, Chem. Commun., 2019, 55, 8398 DOI: 10.1039/C9CC04336E

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