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Issue 47, 2019
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Orchestrated catalytic double rollover annulation: rapid access to N-enriched cationic and neutral PAHs

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Abstract

Disclosed herein is a rhodium(III)-catalyzed novel one-step back-to-back double rollover annulation on pyridine and pyrazine backbones leading to a structurally and optoelectronically diverse class of nicely decorated multi-ring-fused, extensively π-conjugated, N-enriched PAH molecules by virtue of orchestrated quadruple C–H activation events. Selected N-PAHs have been utilized as potential mitochondria and lysosome markers.

Graphical abstract: Orchestrated catalytic double rollover annulation: rapid access to N-enriched cationic and neutral PAHs

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Supplementary files

Article information


Submitted
08 Apr 2019
Accepted
19 May 2019
First published
20 May 2019

Chem. Commun., 2019,55, 6791-6794
Article type
Communication

Orchestrated catalytic double rollover annulation: rapid access to N-enriched cationic and neutral PAHs

P. Karak, C. Dutta, T. Dutta, A. L. Koner and J. Choudhury, Chem. Commun., 2019, 55, 6791
DOI: 10.1039/C9CC02710F

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