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Issue 10, 2019
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Hydroxyl free radical route to the stable siliceous Ti-UTL with extra-large pores for oxidative desulfurization

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Abstract

A facile and mild method was successfully developed to prepare the stable, highly siliceous Ti-UTL zeolite with extra-large pores. The hydroxyl free radical (˙OH) was introduced for the first time to effectively promote the isomorphous substitution of Si for framework Ge under room temperature and neutral conditions, resulting in a stable titanosilicate with an outstanding catalytic activity for oxidative desulfurization.

Graphical abstract: Hydroxyl free radical route to the stable siliceous Ti-UTL with extra-large pores for oxidative desulfurization

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Article information


Submitted
20 Nov 2018
Accepted
28 Dec 2018
First published
02 Jan 2019

Chem. Commun., 2019,55, 1390-1393
Article type
Communication

Hydroxyl free radical route to the stable siliceous Ti-UTL with extra-large pores for oxidative desulfurization

D. Shi, L. Xu, P. Chen, T. Ma, C. Lin, X. Wang, D. Xu and J. Sun, Chem. Commun., 2019, 55, 1390
DOI: 10.1039/C8CC09225G

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