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Issue 70, 2018
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Single-molecule magnet behaviour in a dysprosium-triradical complex

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Abstract

The first triradical bridged binuclear penta-spin single-molecule magnet, [Dy2(hfac)6(BTR)], based on a nitronyl nitroxide triradical was synthesized and characterized. Theoretical calculations revealed Dy-radical antiferromagnetic coupling and radical–radical ferromagnetic coupling. The SMM behavior is found to originate from the exchange states, rather than the isolated Dy3+ center.

Graphical abstract: Single-molecule magnet behaviour in a dysprosium-triradical complex

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Publication details

The article was received on 13 Jun 2018, accepted on 17 Jul 2018 and first published on 17 Jul 2018


Article type: Communication
DOI: 10.1039/C8CC04739A
Chem. Commun., 2018,54, 9726-9729

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    Single-molecule magnet behaviour in a dysprosium-triradical complex

    Z. Xiao, H. Miao, D. Shao, H. Wei, Y. Zhang and X. Wang, Chem. Commun., 2018, 54, 9726
    DOI: 10.1039/C8CC04739A

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