Two transition metal phosphonate photocatalysts for H2 evolution and CO2 reduction

Jiajia Wang; Ruoqian Zhang; Yuanyuan Liu; Zeyan Wang; Peng Wang; Zhaoke Zheng; Xiaoyan Qin; Xiaoyang Zhang; Ying Dai; Baibiao Huang

doi:10.1039/C8CC02822B

Two transition metal phosphonate photocatalysts for H₂ evolution and CO₂ reduction†

Jiajia Wang,^a Ruoqian Zhang,^a Yuanyuan Liu,

*^a Zeyan Wang,

^a Peng Wang,

^a Zhaoke Zheng,^a Xiaoyan Qin,^a Xiaoyang Zhang,^a Ying Dai

^b and Baibiao Huang

*^a

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* Corresponding authors

^a State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China
E-mail: yyliu@sdu.edu.cn, bbhuang@sdu.edu.cn

^b School of Physics, Shandong University, Jinan 250100, China

Abstract

Two transition metal (Co and Ni) ion phosphonates as isostructural organic inorganic hybrids are prepared and investigated in terms of photocatalytic hydrogen evolution from water and CO₂ reduction under UV light irradiation. A photocatalytic mechanism of ligand-to-metal charge transfer (LMCT) is proposed.

Chemical Communications

Two transition metal phosphonate photocatalysts for H₂ evolution and CO₂ reduction†

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Two transition metal phosphonate photocatalysts for H₂ evolution and CO₂ reduction

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Chemical Communications