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Issue 74, 2017
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Polymer-immobilized, hybrid multi-catalyst architecture for enhanced electrochemical oxidation of glycerol

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Abstract

The development of a hybrid, tri-catalytic architecture is demonstrated by immobilizing MWCNTs, TEMPO-modified linear poly(ethylenimine) and oxalate decarboxylase on an electrode to enable enhanced electrochemical oxidation of glycerol. This immobilized, hybrid catalytic motif results in a synergistic 3.3-fold enhancement of glycerol oxidation and collects up to 14 electrons per molecule of glycerol.

Graphical abstract: Polymer-immobilized, hybrid multi-catalyst architecture for enhanced electrochemical oxidation of glycerol

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Article information


Submitted
24 Jul 2017
Accepted
25 Aug 2017
First published
25 Aug 2017

Chem. Commun., 2017,53, 10310-10313
Article type
Communication

Polymer-immobilized, hybrid multi-catalyst architecture for enhanced electrochemical oxidation of glycerol

F. C. Macazo, D. P. Hickey, S. Abdellaoui, M. S. Sigman and S. D. Minteer, Chem. Commun., 2017, 53, 10310
DOI: 10.1039/C7CC05724E

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