Ligand controlled switchable selectivity in ruthenium catalyzed aerobic oxidation of primary amines

Ritwika Ray; Shubhadeep Chandra; Vishal Yadav; Prasenjit Mondal; Debabrata Maiti; Goutam Kumar Lahiri

doi:10.1039/C6CC10200J

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Ligand controlled switchable selectivity in ruthenium catalyzed aerobic oxidation of primary amines†

Ritwika Ray,*^a Shubhadeep Chandra,^a Vishal Yadav,^a Prasenjit Mondal,^a Debabrata Maiti

*^a and Goutam Kumar Lahiri

*^a

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* Corresponding authors

^a Department of Chemistry, Indian Institute of Technology, Bombay, Powai, Mumbai-400076, India
E-mail: ritwika@chem.iitb.ac.in, dmaiti@chem.iitb.ac.in, lahiri@chem.iitb.ac.in

Abstract

A ligand controlled catalytic system for the aerobic oxidation of 1° amines to nitriles and imines has been developed where the varying π-acidic feature of BIAN versus phen in the frameworks of ruthenium catalysts facilitates switchable selectivity.

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DOI: https://doi.org/10.1039/C6CC10200J
Article type: Communication
Submitted: 23 Dec 2016
Accepted: 17 Mar 2017
First published: 17 Mar 2017

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Chem. Commun., 2017,53, 4006-4009

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Ligand controlled switchable selectivity in ruthenium catalyzed aerobic oxidation of primary amines

R. Ray, S. Chandra, V. Yadav, P. Mondal, D. Maiti and G. K. Lahiri, Chem. Commun., 2017, 53, 4006 DOI: 10.1039/C6CC10200J

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Chemical Communications

Ligand controlled switchable selectivity in ruthenium catalyzed aerobic oxidation of primary amines†

Abstract

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Ligand controlled switchable selectivity in ruthenium catalyzed aerobic oxidation of primary amines

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