SCHEDULED MAINTENANCE
A newly developed chiral imidazole nucleophilic catalyst, Acyloxy-DPI, was readily prepared and successfully applied to the enantioselective Black rearrangement with up to 88% ee for a wide range of substrates possessing different substituted groups. A plausible mechanism for the high enantioselectivity was proposed.
M. Wang, Z. Zhang, S. Liu, F. Xie and W. Zhang, Chem. Commun., 2014, 50, 1227 DOI: 10.1039/C3CC47455K
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