Issue 14, 2024
From the journal:

New Journal of Chemistry

Highly enantioselective allylic amination reaction through aerobic oxidative organo–organo dual catalytic system†

Chengli Mou, ORCID logo ‡a   Guangping Liang,‡c   Peiyao Liang,b   Siyi Chen,b   Chong Wu,*a   Shenghan Teng*b  and  Shoulei Wang ORCID logo *b  

* Corresponding authors

a School of Pharmacy, Guizhou University of Traditional Chinese Medicine, Guiyang 550025, China
E-mail: wuchongchem@163.com

b Strait Laboratory of Flexible Electronics (SLoFE), Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Normal University, Fuzhou 350117, China
E-mail: ifeshhteng@fjnu.edu.cn, ifeshlwang@fjnu.edu.cn

c Department of Pharmacy, Zunyi Medical and Pharmaceutical College, Zunyi 563006, China

Abstract

A variety of enantioenriched substituted imides were facilely synthesized through aerobic oxidation/allylic amination reactions of aldimines with MBH carbonates under N-heterocyclic carbene (NHC)/chiral tertiary amine dual catalysis. The strategy is attractive and valuable because of the convenient one-step procedure, environmental friendliness, high enantioselectivity and good functional-group tolerance.

Graphical abstract: Highly enantioselective allylic amination reaction through aerobic oxidative organo–organo dual catalytic system

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Article information

DOI
https://doi.org/10.1039/D4NJ00478G
Article type
Communication
Submitted
29 Jan 2024
Accepted
16 Mar 2024
First published
18 Mar 2024

New J. Chem., 2024,48, 6076-6080

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Highly enantioselective allylic amination reaction through aerobic oxidative organo–organo dual catalytic system

C. Mou, G. Liang, P. Liang, S. Chen, C. Wu, S. Teng and S. Wang, New J. Chem., 2024, 48, 6076 DOI: 10.1039/D4NJ00478G

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