Plasma-catalytic one-step steam reforming of CH4 to CH3OH and H2 promoted by oligomerized [Cu–O–Cu] species on zeolites

Wei Fang; Ximiao Wang; Shangkun Li; Yingzi Hao; Yuping Yang; Wenping Zhao; Rui Liu; Dongxing Li; Chuang Li; Xiaoxia Gao; Li Wang; Hongchen Guo; Yanhui Yi

doi:10.1039/D4GC00265B

Plasma-catalytic one-step steam reforming of CH₄ to CH₃OH and H₂ promoted by oligomerized [Cu–O–Cu] species on zeolites†

Wei Fang,^a Ximiao Wang,^a Shangkun Li,^ab Yingzi Hao,^a Yuping Yang,^a Wenping Zhao,^c Rui Liu,^a Dongxing Li,^a Chuang Li,

^a Xiaoxia Gao,^d Li Wang,^e Hongchen Guo^a and Yanhui Yi

*^a

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* Corresponding authors

^a State Key Laboratory of Fine Chemicals, Frontier Science Center for Smart Materials, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, P.R. China
E-mail: yiyanhui@dlut.edu.cn

^b Research Group PLASMANT, Department of Chemistry, University of Antwerp, Universiteitsplein 1, BE-2610 Wilrijk-Antwerp, Belgium

^c China Tianchen Engineering Corporation, Tianjin, P.R. China

^d Instrumental Analysis Center, Dalian University of Technology, Dalian, P.R. China

^e College of Environmental Sciences and Engineering, Dalian Maritime University, Dalian 116026, Liaoning, China

Abstract

Oligomerized [Cu–O–Cu] species are reported to be efficient in promoting plasma catalytic one-step steam reforming of methane to methanol and hydrogen, achieving 6.8% CH₄ conversion and 73.1% CH₃OH selectivity without CO₂.

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Plasma-catalytic one-step steam reforming of CH₄ to CH₃OH and H₂ promoted by oligomerized [Cu–O–Cu] species on zeolites†

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Plasma-catalytic one-step steam reforming of CH₄ to CH₃OH and H₂ promoted by oligomerized [Cu–O–Cu] species on zeolites

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