Iron homo- and heterobimetallic complexes supported by a symmetrical dinucleating ligand

Pablo Ríos; Matthew S. See; Oscar Gonzalez; Rex C. Handford; Amélie Nicolay; Guodong Rao; R. David Britt; D. Kwabena Bediako; T. Don Tilley

doi:10.1039/D4CC02155J

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Iron homo- and heterobimetallic complexes supported by a symmetrical dinucleating ligand†

Pablo Ríos,

‡^ab Matthew S. See,

‡^bc Oscar Gonzalez,

^b Rex C. Handford,

^b Amélie Nicolay,

^bc Guodong Rao,

^d R. David Britt,

*^d D. Kwabena Bediako

*^b and T. Don Tilley

*^bc

Author affiliations

* Corresponding authors

^a Instituto de Investigaciones Químicas (IIQ), Departamento de Química Inorgánica, Centro de Innovación en Química Avanzada (ORFEO-CINQA), CSIC and Universidad de Sevilla, 41092 Sevilla, Spain

^b Department of Chemistry, University of California Berkeley, Berkeley, USA
E-mail: bediako@berkeley.edu, tdtilley@berkeley.edu

^c Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA

^d Department of Chemistry, University of California, Davis, Davis, California 95616, USA
E-mail: rdbritt@ucdavis.edu

Abstract

The selective synthesis of biomimetic Fe/Mn complexes able to mimic the geometry and catalytic activity of enzymes possessing this cofactor is still a challenge. Herein, we discuss the stepwise synthesis, characterization, and magnetic properties of a Fe(II)/Mn(II) species and related Fe(II)/Fe(II) complexes.

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DOI: https://doi.org/10.1039/D4CC02155J
Article type: Communication
Submitted: 06 May 2024
Accepted: 20 Jul 2024
First published: 22 Jul 2024

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Chem. Commun., 2024,60, 8912-8915

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Iron homo- and heterobimetallic complexes supported by a symmetrical dinucleating ligand

P. Ríos, M. S. See, O. Gonzalez, R. C. Handford, A. Nicolay, G. Rao, R. D. Britt, D. K. Bediako and T. D. Tilley, Chem. Commun., 2024, 60, 8912 DOI: 10.1039/D4CC02155J

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Chemical Communications

Iron homo- and heterobimetallic complexes supported by a symmetrical dinucleating ligand†

Abstract

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Iron homo- and heterobimetallic complexes supported by a symmetrical dinucleating ligand

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