Issue 47, 2024
From the journal:

Chemical Communications

Enabling direct oxidation of ethane to acetaldehyde with oxygen using supported PdO nanoparticles†

Jiajie Ye, ORCID logo ‡a   Shoujie Zhang,‡a   Yanglong Guo, ORCID logo a   Wangcheng Zhan,a   Li Wang,a   Sheng Dai, ORCID logo b   Xuan Tang ORCID logo *ab  and  Yun Guo ORCID logo *a  

* Corresponding authors

a State Key Laboratory of Green Chemical Engineering and Industrial Catalysis, Research Institute of Industrial Catalysis, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, P. R. China
E-mail: xuantang@mail.ecust.edu.cn, yunguo@ecust.edu.cn

b Key Laboratory for Advanced Materials, Feringa Nobel Prize Scientist Joint Research Center, Frontiers Science Center for Materiobiology and Dynamic Chemistry, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, P. R. China

Abstract

Industrial-scale production of acetaldehyde relies heavily on homogeneous catalysts. Here, we used ethane as the feedstock and developed ZSM-5-supported PdO nanoparticles for the direct oxidation of ethane to acetaldehyde by utilizing O2 and CO. PdO nanoparticles clearly demonstrate effective activity and prevent the further deep oxidation of acetaldehyde.

Graphical abstract: Enabling direct oxidation of ethane to acetaldehyde with oxygen using supported PdO nanoparticles

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Article information

DOI
https://doi.org/10.1039/D4CC01734J
Article type
Communication
Submitted
14 Apr 2024
Accepted
14 May 2024
First published
21 May 2024

Chem. Commun., 2024,60, 6067-6070

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Enabling direct oxidation of ethane to acetaldehyde with oxygen using supported PdO nanoparticles

J. Ye, S. Zhang, Y. Guo, W. Zhan, L. Wang, S. Dai, X. Tang and Y. Guo, Chem. Commun., 2024, 60, 6067 DOI: 10.1039/D4CC01734J

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