Carbon defects promoting syngas into liquid fuels over Fe3C@C catalysts

Zhiyuan Fu; Dan Luo; Lei Chen; Yuxue Wei; Mingyang Ren; Wenjing Wang; Chenghua Zhang; Song Sun

doi:10.1039/D3CY00213F

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Carbon defects promoting syngas into liquid fuels over Fe₃C@C catalysts†

Zhiyuan Fu,^a Dan Luo,^b Lei Chen,

^c Yuxue Wei,

*^a Mingyang Ren,^a Wenjing Wang,

^a Chenghua Zhang

^a and Song Sun

Author affiliations

* Corresponding authors

^a School of Chemistry and Chemical Engineering, Anhui University, Hefei, Anhui 230601, China
E-mail: weiyuxue@ahu.edu.cn

^b Department of Applied Chemistry, Yuncheng University, Yuncheng, Shanxi 044000, China

^c School of Materials Science and Engineering, Hefei University of Technology, Hefei 230009, China

Abstract

Carbon wrapped iron catalysts have been intensively studied in recent years to achieve efficient syngas conversion into high-value-added chemicals. A Fe₃C@C catalyst with defect-rich graphite shell exhibits C₅₊ selectivity of 70.1% and CH₄ selectivity of 9.0% at CO conversion of 55.2%, which can be attributed to the enhanced reactant adsorption and anti-oxidation of Fe₃C during FTS.

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Article information

DOI: https://doi.org/10.1039/D3CY00213F
Article type: Communication
Submitted: 15 Feb 2023
Accepted: 11 Mar 2023
First published: 13 Mar 2023

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Catal. Sci. Technol., 2023,13, 2010-2014

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Carbon defects promoting syngas into liquid fuels over Fe₃C@C catalysts

Z. Fu, D. Luo, L. Chen, Y. Wei, M. Ren, W. Wang, C. Zhang and S. Sun, Catal. Sci. Technol., 2023, 13, 2010 DOI: 10.1039/D3CY00213F

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