Issue 25, 2022

Colloidal clustering and diffusion in a convection cell array

Abstract

We numerically investigated the clustering of a uniform suspension of finite-size disks in a linear array of two-dimensional convection cells. We observed that, due to steric interactions, the disks tend to form coherently rotating spatial structures at the center of each cell, as a combined effect of advection and pair collisions. Micellar, ring-like and hexatic patterns emerge in the deterministic regime, depending on the suspension density, but dissolve in the presence of thermal fluctuations. Moreover, pair collisions suffice to activate cell crossings even by noiseless disks and, therefore, cause athermal diffusion. The robustness of such collision induced effects is studied against the opposing action of thermal noise, transverse biases, and particle self-propulsion.

Graphical abstract: Colloidal clustering and diffusion in a convection cell array

Article information

Article type
Paper
Submitted
21 Apr 2022
Accepted
26 May 2022
First published
02 Jun 2022

Soft Matter, 2022,18, 4778-4785

Colloidal clustering and diffusion in a convection cell array

Y. Li, Y. Zhou, F. Marchesoni and P. K. Ghosh, Soft Matter, 2022, 18, 4778 DOI: 10.1039/D2SM00500J

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