Phosphate anion-induced silver-chalcogenide cluster-based metal organic frameworks as dual-functional catalysts for detoxifying chemical warfare agent simulants

Chun-Hua Gong; Zhi-Bing Sun; Man Cao; Xi-Ming Luo; Jie Wu; Qian-You Wang; Shuang-Quan Zang; Thomas C. W. Mak

doi:10.1039/D2CC03120E

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Phosphate anion-induced silver-chalcogenide cluster-based metal organic frameworks as dual-functional catalysts for detoxifying chemical warfare agent simulants†

Chun-Hua Gong,^a Zhi-Bing Sun,^a Man Cao,^a Xi-Ming Luo,

^a Jie Wu,

^a Qian-You Wang,

*^a Shuang-Quan Zang

*^a and Thomas C. W. Mak

^ab

Author affiliations

* Corresponding authors

^a Henan Key Laboratory of Crystalline Molecular Functional Materials, Henan International Joint Laboratory of Tumor Theranostical Cluster Materials, Green Catalysis Center, and College of Chemistry, Zhengzhou University, Zhengzhou 450001, China
E-mail: zangsqzg@zzu.edu.cn

^b Department of Chemistry, The Chinese University of Hong Kong, Hong Kong SAR 999077, China

Abstract

Two porphyrinic silver-chalcogenide cluster-based MOFs were achieved using a phosphate anionic template strategy, and the highly photoactive organic building modules combined with Lewis acidic silver clusters allow both SCC-MOFs to be used as versatile catalysts for the simultaneous degradation of sulfur mustard and nerve agent simulants.

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DOI: https://doi.org/10.1039/D2CC03120E
Article type: Communication
Submitted: 02 Jun 2022
Accepted: 05 Aug 2022
First published: 08 Aug 2022

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Chem. Commun., 2022,58, 9806-9809

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Phosphate anion-induced silver-chalcogenide cluster-based metal organic frameworks as dual-functional catalysts for detoxifying chemical warfare agent simulants

C. Gong, Z. Sun, M. Cao, X. Luo, J. Wu, Q. Wang, S. Zang and T. C. W. Mak, Chem. Commun., 2022, 58, 9806 DOI: 10.1039/D2CC03120E

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Chemical Communications

Phosphate anion-induced silver-chalcogenide cluster-based metal organic frameworks as dual-functional catalysts for detoxifying chemical warfare agent simulants†

Abstract

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Phosphate anion-induced silver-chalcogenide cluster-based metal organic frameworks as dual-functional catalysts for detoxifying chemical warfare agent simulants

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