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Issue 16, 2021
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An organophotoredox-catalyzed C(sp2)–N cross coupling reaction of cyclic aldimines with cyclic aliphatic amines

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Abstract

An organophotocatalyzed C(sp2)–H/N–H cross-dehydrogenative coupling of cyclic aldimines with aliphatic amines has been developed, which represents the first example of visible-light-induced C–H amination of N-sulfonylated imines. This methodology enables the streamline assembly of amine derivatives via radical mediated C–N bond formation. The current protocol features transition-metal-free, mild conditions, good functional group tolerance and good yields.

Graphical abstract: An organophotoredox-catalyzed C(sp2)–N cross coupling reaction of cyclic aldimines with cyclic aliphatic amines

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Article information


Submitted
04 Feb 2021
Accepted
23 Mar 2021
First published
24 Mar 2021

Org. Biomol. Chem., 2021,19, 3595-3600
Article type
Communication

An organophotoredox-catalyzed C(sp2)–N cross coupling reaction of cyclic aldimines with cyclic aliphatic amines

X. Liu, J. Wang, Z. Wu, F. Li, K. Gao, F. Peng, J. Wang, R. Shen, Y. Zhou and L. Liu, Org. Biomol. Chem., 2021, 19, 3595
DOI: 10.1039/D1OB00223F

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