Construction of hierarchical-porous metal–organic frameworks through esterification reaction for efficient catalysis

Peng Wang; Peng Zhang; Yu Shen; Liu Wang; Hongfeng Li; Wenlei Zhang; Zhida Gu; Xinglong Zhang; Yu Fu; Weina Zhang; Fengwei Huo

doi:10.1039/D1CC03059K

Construction of hierarchical-porous metal–organic frameworks through esterification reaction for efficient catalysis†

Peng Wang,‡^ab Peng Zhang,‡^a Yu Shen,‡^a Liu Wang,^a Hongfeng Li,^a Wenlei Zhang,^b Zhida Gu,^b Xinglong Zhang,^a Yu Fu,

*^b Weina Zhang*^a and Fengwei Huo

*^a

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* Corresponding authors

^a Key Laboratory of Flexible Electronics (KLOFE) & Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech), 30 South Puzhu Road, Nanjing 211816, China
E-mail: iamwnzhang@njtech.edu.cn, iamfwhuo@njtech.edu.cn

^b College of Science, Northeastern University, Shenyang 100819, China
E-mail: fuyu@mail.neu.edu.cn

Abstract

A solvent-assisted strategy was proposed by controlling the coordination equilibrium to fabricate hierarchical-porous metal–organic frameworks (HP-MOFs). The obtained HP-MOFs showed remarkable enhancement in catalytic efficiency in Lewis acid catalysis resulting from the joint efforts of the hierarchical pores and the exposed metal clusters.

Chemical Communications

Construction of hierarchical-porous metal–organic frameworks through esterification reaction for efficient catalysis†

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Construction of hierarchical-porous metal–organic frameworks through esterification reaction for efficient catalysis

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