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Electrochemical oxidative C–H/S–H cross-coupling between enamines and thiophenols with H2 evolution

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Abstract

Electrochemical oxidative C–H/S–H cross-coupling has been developed to construct the C–S bond in a highly straightforward and efficient manner. Various enamines and (hetero)aryl thiols could be transformed smoothly under undivided electrolytic cell conditions. Moreover, this electrosynthesis strategy not only avoided the use of chemical oxidants and transition metal catalysts, but also exhibited excellent atom economy.

Graphical abstract: Electrochemical oxidative C–H/S–H cross-coupling between enamines and thiophenols with H2 evolution

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Publication details

The article was received on 17 Nov 2018, accepted on 05 Jan 2019 and first published on 18 Jan 2019


Article type: Edge Article
DOI: 10.1039/C8SC05143G
Citation: Chem. Sci., 2019, Advance Article
  • Open access: Creative Commons BY-NC license
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    Electrochemical oxidative C–H/S–H cross-coupling between enamines and thiophenols with H2 evolution

    D. Li, S. Li, C. Peng, L. Lu, S. Wang, P. Wang, Y. Chen, H. Cong and A. Lei, Chem. Sci., 2019, Advance Article , DOI: 10.1039/C8SC05143G

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