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Surface Modification of Self-Assembled Isoporous Polymer Membranes for Pressure-Dependent High-Resolution Separation

Abstract

Polymer membranes with narrow pore size distribution have received considerable attention because of the high-resolution and high-efficiency separation performance. By elaborately adjusting the parameters in the membrane formation process, we fabricated self-assembled perforated membranes with a series of pore diameters via the breath figure method. The membranes have very narrow pore size distribution and can be considered isoporous membranes. Membranes with controllable surface chemistry were further achieved by the dopamine chemistry. The separation performance of the membranes was systematically investigated under different external pressures. We found that yeast cells can pass through membranes with a pore diameter smaller than the cell size under relatively high operation pressure. The isoporous membranes were also applied to the separation of cell mixtures such as yeasts and lactobacilli. A very high flux is obtained under a pressure of as low as 0.004 MPa. Moreover, yeast cells are completely separated from lactobacilli with a rejection ratio of about 100%. The self-assembled isoporous membranes can also be applied in other size-based separation systems with excellent separation performance and reusability, enabling new opportunities in fields such as bio-separation and biosensors.

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Supplementary files

Publication details

The article was accepted on 14 May 2019 and first published on 15 May 2019


Article type: Paper
DOI: 10.1039/C9PY00560A
Polym. Chem., 2019, Accepted Manuscript

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    Surface Modification of Self-Assembled Isoporous Polymer Membranes for Pressure-Dependent High-Resolution Separation

    Y. Ou, D. Zhou, Z. Xu and L. Wan, Polym. Chem., 2019, Accepted Manuscript , DOI: 10.1039/C9PY00560A

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