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Issue 24, 2019
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Si1−xGex nanoantennas with a tailored Raman response and light-to-heat conversion for advanced sensing applications

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Abstract

Active light-emitting all-dielectric nanoantennas recently have demonstrated great potential as highly efficient nanoscale light sources owing to their strong luminescent and Raman responses. However, their large-scale fabrication faces a number of problems related to productivity limits of existing lithography techniques. Thus, high-throughput fabrication strategies allowing in a facile way to tailor of the nanoantenna emission and thermal properties in the process of their fabrication are highly desirable for various applications. Here, we propose a cost-effective approach to large-scale fabrication of Si1−xGex alloyed Mie nanoresonators possessing an enhanced inherent Raman response which can be simply tailored via tuning the Ge concentration. Moreover, by tailoring the relative Ge composition one can gradually change a complex refractive index of the produced Si1−xGex alloy, which affects the ratio between radiative and nonradiative losses in Si1−xGex nanoantennas, which is crucial for optimization of their optical heating efficiency. Composition-tunable Si1−xGex nanoantennas with an optimized size, light-to-heat conversion and Raman response are implemented for non-invasive sensing of 4-aminothiophenol molecules with a temperature feedback modality and high subwavelength spatial resolution. The results are important for advanced multichannel optical sensing, providing information on analyte's composition, analyte-nanoantenna temperature response and spatial position.

Graphical abstract: Si1−xGex nanoantennas with a tailored Raman response and light-to-heat conversion for advanced sensing applications

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Publication details

The article was received on 01 Mar 2019, accepted on 26 Mar 2019 and first published on 01 Apr 2019


Article type: Paper
DOI: 10.1039/C9NR01837A
Nanoscale, 2019,11, 11634-11641

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    Si1−xGex nanoantennas with a tailored Raman response and light-to-heat conversion for advanced sensing applications

    E. Mitsai, M. Naffouti, T. David, M. Abbarchi, L. Hassayoun, D. Storozhenko, A. Mironenko, S. Bratskaya, S. Juodkazis, S. Makarov and A. Kuchmizhak, Nanoscale, 2019, 11, 11634
    DOI: 10.1039/C9NR01837A

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