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Stereospecific assembly of tetrahydroquinolines via tandem ring-opening/oxidative cyclization of donor-acceptor cyclopropanes with N-alkyl anilines

Abstract

Aerobic copper-catalyzed tandem reaction of N-alkyl anilines with donor-acceptor cyclopropanes is presented for the construction of tetrahydroquinolines via a sequential stereospecific ring opening and oxidative cyclization. The catalyst plays a dual role as a Lewis acid as well as redox catalyst. Air as an oxidant and broad substrate scope are the important practical features.

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Publication details

The article was received on 25 May 2019, accepted on 11 Jun 2019 and first published on 12 Jun 2019


Article type: Communication
DOI: 10.1039/C9CC04042K
Chem. Commun., 2019, Accepted Manuscript

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    Stereospecific assembly of tetrahydroquinolines via tandem ring-opening/oxidative cyclization of donor-acceptor cyclopropanes with N-alkyl anilines

    T. Punniyamurthy, B. K. Das and S. Pradhan, Chem. Commun., 2019, Accepted Manuscript , DOI: 10.1039/C9CC04042K

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