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Issue 34, 2016
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Water oxidation catalyzed by molecular di- and nonanuclear Fe complexes: importance of a proper ligand framework

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Abstract

The synthesis of two molecular iron complexes, a dinuclear iron(III,III) complex and a nonanuclear iron complex, based on the dinucleating ligand 2,2′-(2-hydroxy-5-methyl-1,3-phenylene)bis(1H-benzo[d]imidazole-4-carboxylic acid) is described. The two iron complexes were found to drive the oxidation of water by the one-electron oxidant [Ru(bpy)3]3+.

Graphical abstract: Water oxidation catalyzed by molecular di- and nonanuclear Fe complexes: importance of a proper ligand framework

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Publication details

The article was received on 21 Apr 2016, accepted on 10 May 2016 and first published on 24 May 2016


Article type: Communication
DOI: 10.1039/C6DT01554A
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Citation: Dalton Trans., 2016,45, 13289-13293
  • Open access: Creative Commons BY-NC license
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    Water oxidation catalyzed by molecular di- and nonanuclear Fe complexes: importance of a proper ligand framework

    B. Das, B. Lee, E. A. Karlsson, T. Åkermark, A. Shatskiy, S. Demeshko, R. Liao, T. M. Laine, M. Haukka, E. Zeglio, A. F. Abdel-Magied, P. E. M. Siegbahn, F. Meyer, M. D. Kärkäs, E. V. Johnston, E. Nordlander and B. Åkermark, Dalton Trans., 2016, 45, 13289
    DOI: 10.1039/C6DT01554A

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