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Issue 28, 2015
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The first asymmetric total synthesis of lycoposerramine-R

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Abstract

The first asymmetric total synthesis of lycoposerramine-R, a Lycopodium alkaloid possessing a novel skeleton, was accomplished by a strategy featuring the stereoselective intramolecular aldol cyclization giving a cis-fused 5/6 bicyclic skeleton and a new method for the construction of the pyridone ring via the aza-Wittig reaction.

Graphical abstract: The first asymmetric total synthesis of lycoposerramine-R

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Article information


Submitted
24 Apr 2015
Accepted
09 Jun 2015
First published
09 Jun 2015

Org. Biomol. Chem., 2015,13, 7762-7771
Article type
Paper
Author version available

The first asymmetric total synthesis of lycoposerramine-R

H. Ishida, S. Kimura, N. Kogure, M. Kitajima and H. Takayama, Org. Biomol. Chem., 2015, 13, 7762
DOI: 10.1039/C5OB00827A

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