Issue 11, 2014
From the journal:

Journal of Materials Chemistry A

Creation of Brønsted acid sites on Sn-based solid catalysts for the conversion of biomass†

Liang Wang,a   Jian Zhang,a   Xuefeng Wang,bg   Bingsen Zhang,d   Weijie Ji,e   Xiangju Meng,a   Jixue Li,f   Dang Sheng Su,*cd   Xinhe Bao*b  and  Feng-Shou Xiao*a  

* Corresponding authors

a Key Lab of Applied Chemistry of Zhejiang Province, Zhejiang University, Hangzhou 310028, China
E-mail: fsxiao@zju.edu.cn

b State Key Laboratory for Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Science, Dalian 116023, China
E-mail: xhbao@dicp.ac.cn

c Department of Inorganic Chemistry, Fritz Haber Institute of the Max Planck Society, Berlin 14195, Germany
E-mail: dangsheng@fhi-berlin.mpg.de

d Shenyang National Laboratory of Materials Science Institute of Metal Research, Chinese Academy of Science, Shenyang 110016, China

e Key Laboratory of Mesoscopic Chemistry, MOE, Department of Chemistry, Nanjing University, Nanjing 210093, China

f Department of Materials Science and Engineering, Zhejiang University, Hangzhou 310028, China

g School of Environment and Chemical Engeering, Dalian University, Dalian 116622, China

Abstract

Hydroxyl-attached Sn species are highly dispersed on the surface of mesoporous silica (SBA-15) by the grafting of dimethyldichlorostannane followed by calcination to transform the methyl groups into hydroxyl groups (S–Sn–OH). S–Sn–OH has both Lewis and Brønsted acidic sites, resulting in superior catalytic activities in the acetalisation of glycerol.

Graphical abstract: Creation of Brønsted acid sites on Sn-based solid catalysts for the conversion of biomass

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Article information

DOI
https://doi.org/10.1039/C3TA14982J
Article type
Communication
Submitted
02 Dec 2013
Accepted
19 Dec 2013
First published
19 Dec 2013

J. Mater. Chem. A, 2014,2, 3725-3729

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Creation of Brønsted acid sites on Sn-based solid catalysts for the conversion of biomass

L. Wang, J. Zhang, X. Wang, B. Zhang, W. Ji, X. Meng, J. Li, D. S. Su, X. Bao and F. Xiao, J. Mater. Chem. A, 2014, 2, 3725 DOI: 10.1039/C3TA14982J

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