Issue 11, 2014
From the journal:

Physical Chemistry Chemical Physics

Delayed electron–hole pair recombination in iron(iii)-oxo metal–organic frameworks†

Katrien G. M. Laurier,a   Eduard Fron,a   Pedro Atienzar,b   Koen Kennes,a   Hermenegildo Garcia,b   Mark Van der Auweraer,a   Dirk E. De Vos,c   Johan Hofkensa  and  Maarten B. J. Roeffaers*ac  

* Corresponding authors

a Department of Chemistry, KU Leuven, Celestijnenlaan 200F, Heverlee, Belgium

b Instituto de Tecnología Química, Universidad Politécnica Valencia, Camino de Vera s/n, 46022 Valencia, Spain

c Department of Microbial and Molecular Systems, KU Leuven, KasteelparkArenberg 23, Heverlee, Belgium
E-mail: maarten.roeffaers@biw.kuleuven.be
Fax: +32 16 327990
Tel: +32 16 327920

Abstract

The photodynamic properties of a series of Fe(III)-MOFs have been examined via redox reactions with N,N,N′,N′-tetramethyl-p-phenylenediamine as an electron donor and methyl viologen as an electron acceptor. Furthermore, photogeneration of long-lived species in MIL-88B(Fe) has been proven via transient absorption spectroscopy.

Graphical abstract: Delayed electron–hole pair recombination in iron(iii)-oxo metal–organic frameworks

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Article information

DOI
https://doi.org/10.1039/C3CP55028A
Article type
Communication
Submitted
29 Nov 2013
Accepted
21 Jan 2014
First published
22 Jan 2014

Phys. Chem. Chem. Phys., 2014,16, 5044-5047

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Delayed electron–hole pair recombination in iron(III)-oxo metal–organic frameworks

K. G. M. Laurier, E. Fron, P. Atienzar, K. Kennes, H. Garcia, M. Van der Auweraer, D. E. De Vos, J. Hofkens and M. B. J. Roeffaers, Phys. Chem. Chem. Phys., 2014, 16, 5044 DOI: 10.1039/C3CP55028A

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