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Issue 51, 2014
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Inter/intramolecular Cherenkov radiation energy transfer (CRET) from a fluorophore with a built-in radionuclide

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Abstract

The Cherenkov radiation (CR) from [18F]-FDG, [177Lu]-LuCl3 and [90Y]-YCl3 was detected and CR energy transfer (CRET) to several fluorophores was examined. Subsequent fluorescence emission was found to be a function of the position of absorption bands with respect to the CR peak, energy of emitted particles, radionuclide/fluorophore loading, and fluorophore brightness. A variant of the best fluorophore with a built-in radionuclide was synthesized to achieve inter- and intra-molecular CRET.

Graphical abstract: Inter/intramolecular Cherenkov radiation energy transfer (CRET) from a fluorophore with a built-in radionuclide

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Supplementary files

Article information


Submitted
05 Mar 2014
Accepted
01 Apr 2014
First published
01 Apr 2014

Chem. Commun., 2014,50, 6711-6713
Article type
Communication
Author version available

Inter/intramolecular Cherenkov radiation energy transfer (CRET) from a fluorophore with a built-in radionuclide

Y. Bernhard, B. Collin and R. A. Decréau, Chem. Commun., 2014, 50, 6711
DOI: 10.1039/C4CC01690D

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