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Volume 151, 2011
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In situ powder neutron diffraction study of non-stoichiometric phase formation during the hydrogenation of Li3N

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Abstract

The hydrogenation of Li3N at low chemical potential has been studied in situ by time-of-flight powder neutron diffraction and the formation of a non-stoichiometric Li4−2xNH phase and Li4NH observed. The results are interpreted in terms of a model for the reaction pathway involving the production of Li4NH and Li2NH, which subsequently react together to form Li4−2xNH. Possible mechanisms for the production of Li4NH from the hydrogenation of Li3N are discussed.

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Publication details

The article was received on 14 Dec 2010, accepted on 01 Feb 2011 and first published on 21 Jun 2011


Article type: Paper
DOI: 10.1039/C0FD00020E
Citation: Faraday Discuss., 2011,151, 263-270
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    In situ powder neutron diffraction study of non-stoichiometric phase formation during the hydrogenation of Li3N

    D. J. Bull, N. Sorbie, G. Baldissin, D. Moser, M. T. F. Telling, R. I. Smith, D. H. Gregory and D. K. Ross, Faraday Discuss., 2011, 151, 263
    DOI: 10.1039/C0FD00020E

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