Issue 14, 2011
From the journal:

Chemical Communications

An easily accessible Re-based catalyst for the selective conversion of methanol: evidence for an unprecedented active site structure through combined operando techniques†

Anthony Yoboué,ab   Audrey Susset,ab   Asma Tougerti,ab   Daniel Gallego,ab   Sudarsan Venkat Ramani,ab   Malathi Kalyanikar,ab   Dmitriy S. Dolzhnikov,ab   Sileshi G. Wubshet,ab   Yilun Wang,ab   Sylvain Cristol,ab   Valérie Briois,cd   Camille La Fontaine,c   Régis. M. Gauvin,abd   Jean-François Paulab  and  Elise Berrier*abd  

* Corresponding authors

a Université Lille-Nord de France, 59000 Lille, France

b Unité de Catalyse et de Chimie du Solide, Bât. C3 Cité Scientifique Université Lille 1, 59655 Villeneuve d'Ascq Cedex, France
E-mail: Elise.Berrier@univ-lille1.fr
Fax: +33 3 20 45 65 61
Tel: +33 3 20 43 49 47

c SAMBA Beamline, Synchrotron SOLEIL, Saint Aubin, 91190 Gif s/Yvette, France

d CNRS, Centre National de la Recherche Scientifique, France

Abstract

Heterogeneous Re/SiO2 catalysts prepared using a one pot sol–gel synthesis were found to display high activity in the direct, selective methanol conversion to methylal, which is correlated to an unprecedented rhenium oxide structure.

Graphical abstract: An easily accessible Re-based catalyst for the selective conversion of methanol: evidence for an unprecedented active site structure through combined operando techniques

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Article information

DOI
https://doi.org/10.1039/C0CC05542E
Article type
Communication
Submitted
13 Dec 2010
Accepted
08 Feb 2011
First published
01 Mar 2011

Chem. Commun., 2011,47, 4285-4287

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An easily accessible Re-based catalyst for the selective conversion of methanol: evidence for an unprecedented active site structure through combined operando techniques

A. Yoboué, A. Susset, A. Tougerti, D. Gallego, S. V. Ramani, M. Kalyanikar, D. S. Dolzhnikov, S. G. Wubshet, Y. Wang, S. Cristol, V. Briois, C. La Fontaine, Régis. M. Gauvin, J. Paul and E. Berrier, Chem. Commun., 2011, 47, 4285 DOI: 10.1039/C0CC05542E

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