Issue 18, 2006
From the journal:

Chemical Communications

Electroactive mesoporous tantalum oxidecatalysts for nitrogenactivation and ammonia synthesis†

Chaoyang Yue,a   Michel Trudeaub  and  David Antonelli*a  

* Corresponding authors

a Department of Chemistry and Biochemistry, University of Windsor, 401 Sunset Avenue, Windsor, Ontario, Canada
E-mail: danton@uwindsor.ca
Fax: +1(519) 973-7098

b Emerging Technologies, Hydro-Québec Research Institute, 1800 Boul. Lionel-Boulet, Varennes, Quebec, Canada

Abstract

A new mesoporous Ta oxide catalyst for conversion of dinitrogen to ammonia shows strong evidence for a novel mechanism involving low valent Ta on the surface, supporting recent work in organometallic chemistry using low valent early transition metals for dinitrogen cleavage.

Graphical abstract: Electroactive mesoporous tantalum oxide catalysts for nitrogen activation and ammonia synthesis

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Article information

DOI
https://doi.org/10.1039/B517415E
Article type
Communication
Submitted
07 Dec 2005
Accepted
02 Feb 2006
First published
20 Feb 2006

Chem. Commun., 2006, 1918-1920

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Electroactive mesoporous tantalum oxide catalysts for nitrogen activation and ammonia synthesis

C. Yue, M. Trudeau and D. Antonelli, Chem. Commun., 2006, 1918 DOI: 10.1039/B517415E

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