One parameter fs-pulse form control on NaK and Na2K
Abstract
One parameter control experiments are carried out on two simple model systems with different complexities, the dimer NaK and the trimer Na2K. The influence of the most important pulse features in formally found optimal control results are investigated independently for both molecules: the chirp and the separation of subpulses in pulse trains. For both molecules, the photoinduced processes under control are the transient three