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Experimental and theoretical studies show that H2 reacts with an Ir phosphine complex having a basic pendant amino group to give either an H2 or an Ir–H···H–N hydrogen-bonded hydride complex, depending on the basicity of the phosphine ligands.
D. Lee, B. P. Patel, R. H. Crabtree, E. Clot and O. Eisenstein, Chem. Commun., 1999, 297 DOI: 10.1039/A808601J
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