The use of inelastic neutron scattering spectroscopy has enabled all the internal and external modes of K2MCl6 (M=Pt, Ir) to be observed and assigned for the first time. Based on the results, a reliable, empirical forcefield has been developed. Comparison with forcefields in the literature show that previously they all suffered from using an incomplete set of frequencies.
S. F. Parker and J. Bruce Forsyth, J. Chem. Soc., Faraday Trans., 1998, 94, 1111 DOI: 10.1039/A709215F
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