A series of amine donor-substituted dicyanoquinodimethane molecules with large calculated hyperpolarizabilities has been investigated. Molecular and crystal structure details of a prototypical system are presented. Moderate to strong phase-matched powder second-harmonic generation is observed in chiral amine-substituted compounds.
M. Ravi, D. N. Rao, S. Cohen, I. Agranat and T. P. Radhakrishnan, J. Mater. Chem., 1996, 6, 1119 DOI: 10.1039/JM9960601119
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