Concise enantiospecific synthesis of the key intermediate for ajmalicine 1 and 19-epi-ajmalicine 2 has been achieved starting from a chiral cyclopentanone derivative, easily derived from (–)-carvone.
T. Honda, N. Haze, H. Ishige, K. Masuda, K. Naito and Y. Suzuki, J. Chem. Soc., Perkin Trans. 1, 1993, 539 DOI: 10.1039/P19930000539
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