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Ab initio molecular orbital theory suggests that the non-tetrahedral structural features of the prototype carbenoid, CH2LiF, are retained in its dimer; however, dissociation of singlet methylene is thermodynamically much more favourable from the dimer than from the monomer.
C. Rohde, T. Clark, E. Kaufmann and P. von Ragué Schleyer, J. Chem. Soc., Chem. Commun., 1982, 882 DOI: 10.1039/C39820000882
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