The X-band e.s.r. spectra of Gd3+ doped into single crystals of Na3[La(C7H3NO4)3}·15H2O and into La{N(SiMe3)2]3 are reported and interpreted in terms of the same spin Hamiltonian. The zero-field splitting of 4.66 cm–1 obtained for Gd[N(SiMe3)2]3 appears to be the largest yet reported for Gd3+.
D. S. Katoch and K. D. Sales, J. Chem. Soc., Dalton Trans., 1980, 2476 DOI: 10.1039/DT9800002476
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