Spiro-compounds with silicon and phosphorus as central atoms have been studied using semiempirical molecular orbital calculations. The inclusion of 3d orbitals causes a considerable increase of the split between the anti-bonding b1 and a2 orbitals.
M. C. Böhm and R. Gleiter, J. Chem. Soc., Perkin Trans. 2, 1979, 443 DOI: 10.1039/P29790000443
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